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  4. Stephan Götzinger

Prof. Stephan Götzinger

  • Professor
  • Room: A.3.230
  • Telephone: +49 9131 7133315
  • E-mail

My research is focused on solid-state quantum optics. In the past few years I have, for example, investigated methods to collect single photons with near-unity efficiency. Another emphasis is on techniques which can be used to enhance the interaction of a single photon with a single emitter.

2016

Few-photon coherent nonlinear optics with a single molecule

Andreas Maser, Benjamin Gmeiner, Tobias Utikal, Stephan Goetzinger, Vahid Sandoghdar

Nature Photonics 10 450-453 (2016) | Journal

The pioneering experiments in linear spectroscopy were performed using flames in the 1800s, but nonlinear optical measurements had to wait until lasers became available in the twentieth century. Because the nonlinear cross-section of materials is very small(1,2), macroscopic bulk samples and pulsed lasers are usually used. Numerous efforts have explored coherent nonlinear signal generation from individual nanoparticles(3-5) or small atomic ensembles(6-8) with millions of atoms. Experiments on a single semiconductor quantum dot have also been reported, albeit with a very small yield(9). Here, we report the coherent nonlinear spectroscopy of a single molecule under continuous-wave single-pass illumination and the switching of a laser beam by on the order of ten pump photons. The sharp molecular transitions and efficient photon-molecule coupling at a tight focus(10) allow for optical switching with less than a handful of pump photons and are thus promising for applications in quantum engineering(11).

Spectroscopy and microscopy of single molecules in nanoscopic channels: spectral behavior vs. confinement depth

Benjamin Gmeiner, Andreas Maser, Tobias Utikal, Stephan Goetzinger, Vahid Sandoghdar

Physical Chemistry Chemical Physics 18 19588-19594 (2016) | Journal

We perform high-resolution spectroscopy and localization microscopy to study single dye molecules confined to nanoscopic dimensions in one direction. We provide the fabrication details of our nanoscopic glass channels and the procedure for filling them with organic matrices. Optical data on hundreds of molecules in different channel depths show a clear trend from narrow stable lines in deep channels to broader linewidths in ultrathin matrices. In addition, we observe a steady blue shift of the center of the inhomogeneous band as the channels become thinner. Furthermore, we use super-resolution localization microscopy to correlate the positions and orientations of the individual dye molecules with the lateral landscape of the organic matrix, including cracks and strain-induced dislocations. Our results and methodology are useful for a number of studies in various fields such as physical chemistry, solid-state spectroscopy, and quantum nano-optics.

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