We evaluate prospects, performance and temperature limits of a new approach to macroscopic scale laser refrigeration. The considered<br>refrigeration device is based on exciplex-mediated frequency up-conversion inside hollow-core fibers pressurized with a dopant - buffer<br>gas mixture. Exciplexes are excited molecular states formed by two atoms (dopant and buffer) which do not form a molecule in the<br>ground state but exhibit bound states for electronically excited states. The cooling cycle consists of absorption of laser photons during<br>atomic collisions inducing light assisted exciplex formation followed by blue-shifted spontaneous emission on the atomic line of the bare<br>dopant atoms after molecular separation. This process, closely related to reversing the gain mechanism in excimer lasers, allows for a large<br>fraction of collision energy to be extracted in each cycle. The hollow-core fiber plays a crucial role as it allows for strong light-matter<br>interactions over a long distance, which maximizes the cooling rate per unit volume and the cooling efficiency per injected photon while<br>limiting re-absorption of spontaneously emitted photons channeled into unguided radiation modes. Using quantum optical rate equations<br>and refined dynamical simulations we derive general conditions for efficient cooling of both the gas and subsequently of the surrounding<br>solid state environment. Our analytical approach is applicable to any specific exciplex system considered and reveals the shape of the<br>exciplex potential landscapes as well as the density of the dopant as crucial tuning knobs. The derived scaling laws allow for the identification<br>of optimal exciplex characteristics that help to choose suitable gas mixtures that maximize the refrigeration efficiency for specific<br>applications.<br>
Generation of broadband circularly polarized supercontinuum light in twisted photonic crystal fibers
Rafal Sopalla,
Gordon Wong,
Nicolas Joly,
Michael Frosz,
Xin Jiang,
Goran Ahmed,
Philip Russell
We compare the properties of the broadband supercontinuum (SC) generated in twisted and untwisted solid-core photonic crystal fibers when pumped by circularly polarized<br>40 picosecond laser pulses at 1064 nm. In the helically twisted fiber, fabricated by spinning the preform during the draw, the SC is robustly circularly polarized across its entire<br>spectrum whereas, in the straight fiber, axial fluctuations in linear birefringence and polarization-dependent nonlinear effects cause the polarization state to vary randomly with the wavelength. Theoretical modelling confirms the experimental results. Helically twisted photonic crystal fibers permit the generation of pure circularly polarized SC light with excellent polarization stability against fluctuations in input power and environmental perturbations.
Seeded and unseeded high-order parametric down-conversion
Cameron Okoth,
Andrea Cavanna,
Nicolas Joly,
Maria Chekhova
Spontaneous parametric down-conversion (SPDC) has been one of the foremost tools in quantum optics for over five decades. Over that time, it has been used to demonstrate some of the curious features that arise from quantum mechanics. Despite the success of SPDC, its higher-order analogs have never been observed, even though it has been suggested that they generate far more unique and exotic states than SPDC. An example of this is the emergence of non-Gaussian states without the need for postselection. Here we calculate the expected rate of emission for nth-order SPDC with and without external stimulation (seeding). Focusing primarily on third-order parametric down-conversion, we estimate the photon detection rates in a rutile crystal for both the unseeded and seeded regimes.
Scientific career
Since 2021: Head of the microstructured optical fibres independent research group at the Max-Planck Institute for the Science of Light in Erlangen, Germany
Since 2009: Associate professor at the Univ. of Erlangen-Nuremberg in Germany
2005 – 2008: Maître de conférences at the Univ. of Lille in France
Education background
2012: Habilitation at the Ecole Normale Supérieure of Cachan (France) Title: Supercontinuum generation using pulses propagating in photonic crystal fibres, Defended in July. 10th 2012. Thesis adviser: Prof. Dr. Joseph Zyss.
2002-2005: Post-doctoral fellow at the University of Bath (UK) in the group of Prof. Philip Russell
1999-2002: PhD with honors (“Félicitations du jury”) at the laboratory of Physics of Lasers, Atoms, and Molecules (PhLAM) at the University of Lille (France) Title: Instabilities in pulsed mode-locked lasers: techniques for observation and control Defended on Sept. 23rd 2002. Thesis adviser: Prof. Dr. Serge Bielawski.
Awards & appointments
Since 2023: Advisor of the Erlangen Optica Student Chapter
Since 2021: Scientific coordinator of the Internation Max Planck School for the Physics of Light (IMPRS-PL)
Since 2020: Senior member of Optical Society of America (OSA)
Since 2019: Fellow of the Max Planck School of Photonics (MPSP) and member of the selection committee
Since 2016: Fellow of the Max Planck Center for Extreme and Quantum Photonics, Ottawa, Canada
1999: MENRT scholarship from the French ministry of Research to perform his doctoral degree at the University of Lille from 1999 to 2002
1998: Awarded a CIME scholarship from AUF (Agence universitaire de la Francophonie) to perform his Master study at Laval University (Québec) in 1998
Professional activities
2024: Member of the Technical Program Committee for the SPIE Photonics Europe in Strasbourg
Since 2022: Associate Editor of Opt. Express
2017: General chair of the 1st Sino-German symposium on fiber photonics for light-matter interaction in Shanghai, China
2017 – 2018: Member of the Technical Program Committee for SPIE UV and higher energy photonic
2013 – 2017: Member of Technical Program Committee for CLEO US (OSA)
2015: co-Chair of the 2nd Siegman International School of Laser (OSA)
Since 2015: Member of the Technical Program Committee for WSOF (OSA) in Hong-Kong (2015), Limasol in Cypris (2017), Adelaide in Australia (2022), and in Prague in Czech Republic (2025)
Since 20214: Member of the Student Commission of the internation Master of Advanced Optics and Technologies (MAOT)
2013: Topical session at PIERS (Progress in Electromagnetics Research Symposium) in Stockholm
2011: International conference on Nonlinear optics and complexity in photonic crystal fibers and nanostructures in Erice, in Sicily
2011: 14th International SAOT workshop on Fiber laser, sensors and materials at Reicheschwand, Germany
Since 2009: External expert for the evaluation of proposals from ANR (National agency of research in France), the Polish Society of Science, DFG (National agency of research in Germany) and ERC (European Research Council)
Since 2009: Supervisor of 13 PhD students, 2 post-docs, 14 MSc students
Ongoing projects
DFG project JO 1090/8-3 – OrbitFlySens [FAU] Orbiting flying particle sensor (with Bernhard Schmauß, FAU) – 2025-2028
BayFrance FK-34-2024 [FAU] Real-time detection of Terahertz signals using ultrashort lasers Mobility allowance – collaboration with University of Lille - 2025
BayFrance FK-35-2024 [FAU] Exploring chiral fibers for new-type of polarization-resolved endoscopy Mobility allowance – collaboration with University of Marseille – 2025
DFG project JO 1090/3-2 – Photon Triplets [FAU] Generation of photon triplets via three-photon parametric down-conversion (with Maria Chekhova) – 2024-2027
QuNet beta [MPL] 2021-2026
Max-Planck-School of Photonics (MPSP) [FAU] 2019-2025
DFG project JO 1090/6-1 -Twin Beams [FAU] Fiber source of entangled photons with giant tunable frequency separation (with Maria Chekhova) - 2021-2024
DFG project JO 1090/4-1 – Rydbergatoms in photonic crystal fibres [FAU] (with Robert Löw, University of Stuttgart) - 2019-2023
BayFrance FK-29-2018 [FAU] Frequency conversion of single-photon quantum sources using gas-filled hollow-core photonic crystal fibres Mobility allowance – collaboration with LKB, Ens Paris, France - 2018
DFG project JO 1090/3-1 – Photon Triplets [FAU] Generation of photon triplets via three-photon parametric down-conversion (with Maria Chekhova) – 2017-2020
BayFrance FK-38-2013 [FAU] Dynamical instabilities in photonic crystal fiber ring cavities synchronously pumped by femtosecond pulses Mobility allowance – collaboration with University of Lille, France - 2013-2014
