Dr. Claudiu Genes

We provide a fully analytical treatment for the partial refrigeration of the thermal motion of a quantum mechanical resonator under the action of feedback. As opposed to standard cavity optomechanics where the aim is to isolate and cool a single mechanical mode, the aim here is to extract the thermal energy from many vibrational modes within a large frequency bandwidth. We consider a standard cold-damping technique, where homodyne readout of the cavity output field is fed into a feedback loop that provides a cooling action directly applied on the mechanical resonator. Analytical and numerical results predict that low final occupancies are achievable independent of the number of modes addressed by the feedback, as long as the cooling rate is smaller than the intermode frequency separation. For resonators exhibiting a few nearly degenerate pairs of modes, cooling is less efficient and a weak dependence on the number of modes is obtained. These scalings hint toward the design of frequency-resolved mechanical resonators, where efficient refrigeration is possible via simultaneous cold-damping feedback.

We provide a fully analytical treatment for the partial refrigeration of the thermal motion of a quantum mechanical resonator under the action of feedback. As opposed to standard cavity optomechanics where the aim is to isolate and cool a single mechanical mode, the aim here is to extract the thermal energy from many vibrational modes within a large frequency bandwidth. We consider a standard cold-damping technique, where homodyne readout of the cavity output field is fed into a feedback loop that provides a cooling action directly applied on the mechanical resonator. Analytical and numerical results predict that low final occupancies are achievable independent of the number of modes addressed by the feedback, as long as the cooling rate is smaller than the intermode frequency separation. For resonators exhibiting a few nearly degenerate pairs of modes, cooling is less efficient and a weak dependence on the number of modes is obtained. These scalings hint toward the design of frequency-resolved mechanical resonators, where efficient refrigeration is possible via simultaneous cold-damping feedback.

We evaluate prospects, performance and temperature limits of a new approach to macroscopic scale laser refrigeration. The considered<br>refrigeration device is based on exciplex-mediated frequency up-conversion inside hollow-core fibers pressurized with a dopant - buffer<br>gas mixture. Exciplexes are excited molecular states formed by two atoms (dopant and buffer) which do not form a molecule in the<br>ground state but exhibit bound states for electronically excited states. The cooling cycle consists of absorption of laser photons during<br>atomic collisions inducing light assisted exciplex formation followed by blue-shifted spontaneous emission on the atomic line of the bare<br>dopant atoms after molecular separation. This process, closely related to reversing the gain mechanism in excimer lasers, allows for a large<br>fraction of collision energy to be extracted in each cycle. The hollow-core fiber plays a crucial role as it allows for strong light-matter<br>interactions over a long distance, which maximizes the cooling rate per unit volume and the cooling efficiency per injected photon while<br>limiting re-absorption of spontaneously emitted photons channeled into unguided radiation modes. Using quantum optical rate equations<br>and refined dynamical simulations we derive general conditions for efficient cooling of both the gas and subsequently of the surrounding<br>solid state environment. Our analytical approach is applicable to any specific exciplex system considered and reveals the shape of the<br>exciplex potential landscapes as well as the density of the dopant as crucial tuning knobs. The derived scaling laws allow for the identification<br>of optimal exciplex characteristics that help to choose suitable gas mixtures that maximize the refrigeration efficiency for specific<br>applications.<br>

We present a general framework for cavity quantum electrodynamics with strongly frequency-dependent mirrors. The method is applicable to a variety of reflectors exhibiting sharp internal resonances as can be realized, for example, with photonic-crystal mirrors or with two-dimensional atomic arrays around subradiant points. Our approach is based on a modification of the standard input-output formalism to explicitly include the dynamics of the mirror’s internal resonance. We show how to directly extract the interaction parameters from the comparison with classical transfer matrix theory and how to treat the non-Markovian dynamics of the cavity field mode introduced by the mirror’s internal resonance. As an application within optomechanics, we illustrate how a non-Markovian Fano-resonance cavity with a flexible photonic-crystal mirror can provide both sideband resolution as well as strong heating suppression in optomechanical cooling. This approach, amenable to a wide range of systems, opens up possibilities for using hybrid frequency-dependent reflectors in cavity quantum electrodynamics for engineering novel forms of light-matter interactions.

We investigate the interaction between light and molecular systems modeled as quantum emitters coupled to a multitude of vibrational modes via a Holstein-type interaction. We follow a quantum Langevin equations approach that allows for analytical derivations of absorption and fluorescence profiles of molecules driven by classical fields or coupled to quantized optical modes. We retrieve analytical expressions for the modification of the radiative emission branching ratio in the Purcell regime and for the asymmetric cavity transmission associated with dissipative cross talk between upper and lower polaritons in the strong coupling regime. We also characterize the Förster resonance energy transfer process between donor-acceptor molecules mediated by the vacuum or by a cavity mode.

Cavity-embedded quantum emitters show strong modifications of free space radiation properties such as an enhanced decay known as the Purcell effect. The central parameter is the cooperativity C - the ratio of the square of the coherent cavity coupling strength over the product of cavity and emitter decay rates. For a single emitter, C is independent of the transition dipole moment and dictated by geometric cavity properties such as finesse and mode waist. In a recent work Phys. Rev. Lett. 119, 093601 (2017) we have shown that collective excitations in ensembles of dipole-dipole coupled quantum emitters show a disentanglement between the coherent coupling to the cavity mode and spontaneous free space decay. This leads to a strong enhancement of the cavity cooperativity around certain collective subradiant antiresonances. Here, we present a quantum Langevin equations approach aimed at providing results beyond the classical coupled dipoles model. We show that the subradiantly enhanced cooperativity imprints its effects onto the cavity output field quantum correlations while also strongly increasing the cavity-emitter system's collective Kerr nonlinear effect.

The transversely confined propagating modes of an optical fiber mediate virtually infinite range energy exchanges among atoms placed within their field, which adds to the inherent free space dipole–dipole coupling. Typically, the single atom free space decay rate largely surpasses the emission rate into the guided fiber modes. However, scaling up the atom number as well as the system size amounts to entering a collective emission regime, where fiber-induced superradiant spontaneous emission dominates over free space decay. We numerically study this super- and subradiant decay of highly excited atomic states for one or several transverse fiber modes as present in hollow core fibers. As particular excitation scenarios we compare the decay of a totally inverted state to the case of π/2 pulses applied transversely or along the fiber axis as in standard Ramsey or Rabi interferometry. While a mean field approach fails to correctly describe the initiation of superradiance, a second-order approximation accounting for pairwise atom–atom quantum correlations generally proves sufficient to reliably describe superradiance of ensembles from two to a few hundred particles. In contrast, a full account of subradiance requires the inclusion of all higher order quantum correlations. Considering multiple guided modes introduces a natural effective cut-off for the interaction range emerging from the dephasing of different fiber contributions.

Radiation pressure forces in cavity optomechanics allow for efficient cooling of vibrational modes of macroscopic mechanical resonators, the manipulation of their quantum states, as well as generation of optomechanical entanglement. The standard mechanism relies on the cavity photons directly modifying the state of the mechanical resonator. Hybrid cavity optomechanics provides an alternative approach by coupling mechanical objects to quantum emitters, either directly or indirectly via the common interaction with a cavity field mode. While many approaches exist, they typically share a simple effective description in terms of a single force acting on the mechanical resonator. More generally, one can study the interplay between various forces acting on the mechanical resonator in such hybrid mechanical devices. This interplay can lead to interference effects that may, for instance, improve cooling of the mechanical motion or lead to generation of entanglement between various parts of the hybrid device. Here, we provide such an example of a hybrid optomechanical system where an ensemble of quantum emitters is embedded into the mechanical resonator formed by a vibrating membrane. The interference between the radiation pressure force and the mechanically modulated Tavis--Cummings interaction leads to enhanced cooling dynamics in regimes in which neither force is efficient by itself. Our results pave the way towards engineering novel optomechanical interactions in hybrid optomechanical systems.