We report, for the first time, the observation of spontaneous parametric down-conversion (SPDC) free of phase matching (momentum conservation).We alleviate the need to conserve momentum by exploiting the<br>position-momentum uncertainty relation and using a planar geometry source, a 6 μm thick layer of lithium niobate. Nonphase-matched SPDC opens up a new platform on which to investigate fundamental quantum<br>effects but it also has practical applications. The ultrasmall thickness leads to a frequency spectrum an order of magnitude broader than that of phase-matched SPDC. The strong two-photon correlations are still<br>preserved due to energy conservation. This results in ultrashort temporal correlation widths and huge frequency entanglement. The studies we make here can be considered as the initial steps into the emerging field of nonlinear quantum optics on the microscale and nanoscale.
Detection-device-independent verification of nonclassical light
M Bohmann,
L Qi,
W Vogel,
Maria Chekhova
Physical Review Research
1
033178
(2019)
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The efficient certification of nonclassical effects of light forms the basis for applications in optical quantum technologies. We derive general correlation conditions for the verification of nonclassical light based on multiplexed detection. The obtained nonclassicality criteria are valid for imperfectly balanced multiplexing scenarios with on-off detectors and do not require any knowledge about the detector system. In this sense, they are fully independent of the detector system. In our experiment, we study light emitted by clusters of single-photon emitters, whose photon number may exceed the number of detection channels. Even under such conditions, our criteria certify nonclassicality with high statistical significance.
Feasibility of quantum key distribution with macroscopically bright coherent light
Olena Kovalenko,
Kirill Spasibko,
M. V. Chekhova,
Vladyslav C. Usenko,
Radim Filip
We address feasibility of continuous-variable quantum key distribution using bright multimode coherent states of light and homodyne detection. We experimentally verify the possibility to properly select signal modes by matching them with the local oscillator and this way to decrease the quadrature noise concerned with unmatched bright modes. We apply the results to theoretically predict the performance of continuous-variable quantum key distribution scheme using multimode coherent states in scenarios where modulation is applied either to all the modes or only to the matched ones, and confirm that the protocol is feasible at high overall brightness. Our results open the pathway towards full-scale implementation of quantum key distribution using bright light, thus bringing quantum communication closer to classical optics.
Experimental reconstruction of spatial Schmidt modes for a wide-field SU(1,1) interferometer
Gaetano Frascella,
Roman V Zakharov,
Olga V Tikhonova,
Maria Chekhova
We study the spatial mode content at the output of a wide-field SU(1, 1) interferometer, i.e. a nonlinear interferometer comprising two coherently-pumped spatially-multimode optical parametric amplifiers placed in sequence with a focusing element in between. This device is expected to provide a phase sensitivity below the shot-noise limit for multiple modes over<br>a broad angular range. To reconstruct the spatial modes and their weights, we implement<br>a simple method based on the acquisition of only intensity distributions. The eigenmode decomposition of the field is obtained through the measurement of the covariance of intensities at different spatial points. We investigate both the radial and azimuthal (orbital angular momentum) modes and show that their total number is large enough to enable applications of the interferometer in spatially-resolved phase measurements.
Nonlinear Mach–Zehnder interferometer with ultrabroadband squeezed light
D. B. Horoshko,
M. I. Kolobov,
F. Gumpert,
I. Shand,
F. König,
M. V. Chekhova
JOURNAL OF MODERN OPTICS
67
41-48
(2019)
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We study both theoretically and experimentally the interference pattern in a nonlinear Mach–Zehnder interferometer formed by two aperiodically-poled crystals, where broadband squeezed light is generated by both crystals via parametric down-conversion with a common quasi- monochromatic pump. This configuration is important for measuring the squeezing produced by the first crystal and also for measuring a small phase shift introduced by a sample between the crystals. On the basis of the approximate quantum Rosenbluth formula for each crystal we develop an ana- lytic model for the field evolution in the interferometer. We report an experimental observation of the interference fringes, caused by the dispersion of the generated PDC waves in both crystals form- ing the interferometer. We observe a displacement of the interference pattern caused by a sample between the crystals and infer the phase shift within a band of 20 nm. The experimental data are in a good agreement with the predictions of the developed model, up to imperfections of the samples.
Wide-field SU(1,1) interferometer
Gaetano Frascella,
E. E. Mikhailov,
N. Takanashi,
R. V. Zakharov,
O. V. Tikhonova,
Maria Chekhova
An SU(1,1) interferometer uses a sequence of two optical parametric amplifiers for achieving sub-shot-noise sensitivity to a phase shift introduced in between. We present the first realization of a wide-field SU(1,1) interferometer, where the use of a focusing element enables spatially multimode operation within a broad angle. Over this angle, the interference phase is found to be flat. This property is important for the high sensitivity to the phase front disturbance. Further, -4.3 +/- 0.7 dB quadrature squeezing, an essential requirement to the high sensitivity, is experimentally demonstrated for plane-wave modes inside the interferometer. Such an interferometer is useful not only for quantum metrology, but also in remote sensing, enhanced sub-shot-noise imaging, and quantum information processing. (C) 2019 Optical Society of America under the terms of the OSA Open Access Publishing Agreement
Indefinite-Mean Pareto Photon Distribution from Amplified Quantum Noise
Mathieu Manceau,
Kirill Spasibko,
Gerd Leuchs,
Radim Filip,
Maria Chekhova
Extreme events appear in many physics phenomena, whenever the probability distribution has a "heavy tail" differing very much from the equilibrium one. Most unusual are the cases of power-law (Pareto) probability distributions. Among their many manifestations in physics, from "rogue waves" in the ocean to Levy flights in random walks, Pareto dependences can follow very different power laws. For some outstanding cases, the power exponents are less than 2, leading to indefinite values not only for higher moments but also for the mean. Here we present the first evidence of indefinite-mean Pareto distribution of photon numbers at the output of nonlinear effects pumped by parametrically amplified vacuum noise, known as bright squeezed vacuum (BSV). We observe a Pareto distribution with power exponent 1.31 when BSV is used as a pump for supercontinuum generation, and other heavy-tailed distributions (however, with definite moments) when it pumps optical harmonics generation. Unlike in other fields, we can flexibly control the Pareto exponent by changing the experimental parameters. This extremely fluctuating light is interesting for ghost imaging and for quantum thermodynamics as a resource to produce more efficiently nonequilibrium states by single-photon subtraction, the latter of which we demonstrate experimentally.
Separated Schmidt modes in the angular spectrum of biphotons
N. A. Borshchevskaia,
F. Just,
K. G. Katamadze,
Andrea Cavanna,
M. V. Chekhova
Laser Physics Letters
16
085207
(2019)
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We prepared qudits based on angular multimode biphoton states by modulating the pump angular spectrum. The modes were prepared in the Schmidt basis and their intensity distributions did not overlap in space. This allows one to get rid of filtering losses while addressing single modes and to realize a single-shot qudit readout.
Seeded and unseeded high-order parametric down-conversion
Cameron Okoth,
Andrea Cavanna,
Nicolas Joly,
Maria Chekhova
Spontaneous parametric down-conversion (SPDC) has been one of the foremost tools in quantum optics for over five decades. Over that time, it has been used to demonstrate some of the curious features that arise from quantum mechanics. Despite the success of SPDC, its higher-order analogs have never been observed, even though it has been suggested that they generate far more unique and exotic states than SPDC. An example of this is the emergence of non-Gaussian states without the need for postselection. Here we calculate the expected rate of emission for nth-order SPDC with and without external stimulation (seeding). Focusing primarily on third-order parametric down-conversion, we estimate the photon detection rates in a rutile crystal for both the unseeded and seeded regimes.
Study of broadband multimode light via non-phase-matched sum frequency generation
Denis Kopylov,
Kirill Spasibko,
Tatiana Murzina,
Maria Chekhova
New Journal of Physics
21
033024
(2019)
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We propose non-phase-matched sum frequency generation (SFG) as a method for characterizing broadband multimode light. Both the central wavelength and the bandwidth are in this case not limited by the phase matching condition. As an example, we consider bright squeezed vacuum (BSV) generated through high-gain parametric down conversion (PDC). In the spectrum of SFG from BSV, we observe the coherent peak and the incoherent background. We show that the ratio of their widths is equal to the number of frequency modes in BSV, which in the case of low-gain PDC gives the degree of frequency entanglement for photon pairs. By generating the sum frequency in the near-surface region of a nonlinear crystal, we increase the SFG efficiency and get rid of the modulation caused by chromatic dispersion, known as Maker fringes. This allows one to use non-phasematched SFG as a wavelength-independent autocorrelator. Furthermore, we demonstrate efficient non-phase-matched three- and four-frequency summation of broadband multimode light, hardly possible under phase matching. We show that the latter contains the coherent peak while the former does not.
Overcoming inefficient detection in sub-shot-noise absorption measurement and imaging
Eugene Knyazev,
Farid Khalili,
Maria Chekhova
Optics Express
27
(6)
7868-7885
(2019)
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Photon-number squeezing and correlations enable measurement of absorption with an accuracy exceeding that of the shot-noise limit. However, sub-shot noise imaging and sensing based on these methods require high detection efficiency, which can be a serious obstacle if measurements are carried out in “difficult” spectral ranges. We show that this problem can be overcome through the phase-sensitive amplification before detection. Here we propose an experimental scheme of sub-shot-noise imaging with tolerance to detection losses.
A primary radiation standard based on quantum nonlinear optics
Samuel Lemieux,
Enno Giese,
Robert Fickler,
Maria Chekhova,
Robert Boyd
The black body remains the most prominent source of light for absolute radiometry. Its main alternative, synchrotron radiation, requires costly and large facilities. Quantum optics offers a new radiometric source: parametric down-conversion (PDC), a nonlinear optical process, in which pairwise photon correlations enable absolute calibration of photodetectors. Since the emission rate crucially depends on the brightness of the electromagnetic field, quantum-mechanical fluctuations of the vacuum can be seen as a seed of spontaneous PDC, and their amplitude is a natural radiometric standard. Thus, they allow for the calibration of the spectral radiance of light sources by measuring the ratio between seeded and unseeded PDC. Here, we directly use the frequency spectrum of the electromagnetic vacuum to trigger spontaneous PDC and employ the generated light to infer the spectral response of a spectrometer over a broad spectral range. Then, we deduce the absolute quantum efficiency from the spectral shape of PDC in the high-gain regime, without relying on a seed or reference detector. Our results compare well with the ones obtained with a reference lamp, demonstrating a promising primary radiation standard.
Kontakt
Forschungsgruppe Maria Chekhova
Max-Planck-Institut für die Physik des Lichts Staudtstr. 2 91058 Erlangen
