Flying Particle Thermosensor in Hollow-Core Fiber Based on Fluorescence Lifetime Measurements
Jasper Freitag,
Max Koeppel,
Maria N. Romodina,
Nicolas Joly,
Bernhard Schmauß
IEEE Journal of Selected Topics in Quantum Electronics
30
(6)
5600409
(2023)
| Journal
| PDF
Thermosensitive fluorescence lifetime measurements enable accurate thermometry independent of intensity fluctuations along the optical path. Here, we report lifetime-based temperature measurements of a single europium-doped particle optically trapped in an air-filled hollow-core fiber. A frequency-domain fluorescence lifetime measurement setup was integrated into a dual-beam optical trap. The measured apparent lifetime shows a linear temperature dependence of −1.8 µs/K for excitation at 400Hz . The results were repeatable over multiple cooling and heating cycles. In addition to temperature sensing, the influence of the high-power trapping laser on the measured apparent lifetime and fluorescence intensity was investigated. The observed laser-induced particle heating can be exploited to increase the fluorophore's sensitivity and operating range for low-temperature sensing. Fluorescence lifetime measurements of optically trapped particles inside a hollow-core fiber are promising for temperature sensing with micrometer spatial resolution over meter-scale distances.
Performance analysis of tabletop single-pulse terahertz detection at rates up to 1.1 MHz
Nicolas Couture,
Markus Lippl,
Wei Cui,
Angela Gamouras,
Nicolas Joly,
Jean-Michel Ménard
Standard terahertz time-domain spectroscopy uses a relatively slow multidata acquisition process that has hindered the technique’s ability to resolve “fast” dynamics occurring on the microsecond timescale. This timescale, inaccessible to most ultrafast pump-probe techniques, hosts a range of phenomena that has been left unexplored due to a lack of proper real-time monitoring techniques. In this work, chirped-pulse spectral encoding, a photonic time-stretch technique, and high-speed electronics are used to demonstrate time-resolved terahertz detection at a rate up to 1.1 MHz. This configuration relies on a tabletop optical source and a setup able to resolve every terahertz transient generated by the same source. We investigate the performance of this single-pulse terahertz detection system at different acquisition rates in terms of experimental noise, dynamic range, and signal-to-noise ratio. Our results pave the way towards single-pulse terahertz time-domain spectroscopy at arbitrarily fast rates to monitor complex dynamics in real time.
Kontakt
Forschungsgruppe Nicolas Joly
Professur für Photonik Friedrich-Alexander-Universität Erlangen-Nürnberg
und
Max-Planck-Institut für die Physik des Lichts Staudtstr. 2 91058 Erlangen, Germany
