Extreme thermodynamics in nanolitre volumes through stimulated Brillouin–Mandelstam scattering
Andreas Geilen,
Alexandra Popp,
Debavan Das,
Saher Junaid,
Christopher G. Poulton,
Mario Chemnitz,
Christoph Marquardt,
Markus A. Schmidt,
Birgit Stiller
Nature Physics
19
1805-1812
(2023)
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Examining the physical properties of materials—particularly of toxic liquids—under a wide range of thermodynamic states is a challenging problem due to the extreme conditions the material has to experience. Such temperature and pressure regimes, which result in a change in the refractive index and sound velocity, can be accessed by optoacoustic interactions such as Brillouin–Mandelstam scattering. Here we demonstrate the Brillouin–Mandelstam measurements of nanolitre volumes of liquids in extreme thermodynamic regimes. This is enabled by a fully sealed liquid-core optical fibre containing carbon disulfide. Within this waveguide, which exhibits tight optoacoustic confinement and a high Brillouin gain, we are able to conduct spatially resolved measurements of the local Brillouin response, giving us access to a resolved image of the temperature and pressure values along the liquid channel. We measure the material properties of the liquid core at very large positive pressures (above 1,000 bar) and substantial negative pressures (below –300 bar), as well as explore the isobaric and isochoric regimes. The extensive thermodynamic control allows the tunability of the Brillouin frequency shift of more than 40% using only minute volumes of liquid.
Spin-orbit interaction in nanofiber-based Brillouin scattering
Maxime Zerbib,
Maxime Romanet,
Thibaut Sylvestre,
Christian Wolff,
Birgit Stiller,
Jean-Charles Beugnot,
Kien Phan Huy
Optics Express
31
(14)
22284-22295
(2023)
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Angular momentum is an important physical property that plays a key role in light-matter interactions such as spin-orbit interaction. Here, we investigate theoretically and experimentally the spin-orbit interaction between a circularly polarized optical (spin) and a transverse vortex acoustic wave (orbital) using Brillouin backscattering in a silica optical nanofiber. We specifically explore the state of polarization of Brillouin backscattering induced by the TR21 torso-radial vortex acoustic mode that carries an orbital angular momentum. Using a full-vectorial theoretical model, we predict and observe two operating regimes for which the backscattered Brillouin signal is either depolarized or circularly polarized depending on the input pump polarization. We demonstrate that when the pump is circularly polarized and thus carries a spin angular momentum, the backscattered signal undergoes a handedness reversal of circular polarization due to optoacoustic spin-orbit interaction and the conservation of overall angular momentum.
Dynamic Brillouin cooling for continuous optomechanical systems
Changlong Zhu,
Birgit Stiller
Materials for Quantum Technology
3
015003
(2023)
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Up until now, ground state cooling using optomechanical interaction is realized in the regime where optical dissipation is higher than mechanical dissipation. Here, we demonstrate that optomechanical ground state cooling in a continuous optomechanical system is possible by using backward Brillouin scattering while mechanical dissipation exceeds optical dissipation which is the common case in optical waveguides. The cooling is achieved in an anti-Stokes backward Brillouin process by modulating the intensity of the optomechanical coupling via a pulsed pump to suppress heating processes in the strong coupling regime. With such dynamic modulation, a significant cooling factor can be achieved, which can be several orders of magnitude lower than for the steady-state case. This modulation scheme can also be applied to Brillouin cooling generated by forward intermodal Brillouin scattering.
Optical Vortex Brillouin Laser
Xinglin Zeng,
Philip Russell,
Yang Chen,
Zheqi Wang,
Gordon Wong,
Paul Roth,
Michael Frosz,
Birgit Stiller
Optical vortices, which have been extensively studied over the last decades, offer an additional degree of freedom useful in many applications, such as optical tweezers and quantum control. Stimulated Brillouin scattering (SBS), providing a narrow linewidth and a strong nonlinear response, has been used to realize quasi-continuous wave lasers. Here, stable oscillation of optical vortices and acoustic modes in a Brillouin laser based on chiral photonic crystal fiber (PCF) is reported, which robustly supports helical Bloch modes (HBMs) that carry circularly polarized optical vortex and display circular birefringence. A narrow-linewidth Brillouin fiber laser that stably emits 1st- and 2nd-order vortex-carrying HBMs is implemented. Angular momentum conservation selection rules dictate that pump and backward Brillouin signals have opposite topological charge and spin. Additionally, it is shown that when the chiral PCF is placed within a laser ring cavity, the linewidth-narrowing associated with lasing permits the peak of the Brillouin gain that corresponds to acoustic mode to be measured with resolution of 10 kHz and accuracy of 520 kHz. The results pave the way to a new generation of vortex-carrying SBS systems with applications in optical tweezers, quantum information processing, and vortex-carrying nonreciprocal systems.
Quantum coherent control in pulsed waveguide optomechanics
Junyin Zhang,
Changlong Zhu,
Christian Wolff,
Birgit Stiller
Physical Review Research
5
(1)
013010
(2023)
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Coherent control of traveling acoustic excitations in a waveguide system is an interesting way to manipulate and transduce classical and quantum information. So far, these interactions, often based on optomechanical resonators or Brillouin scattering, have been studied in the steady-state regime using continuous waves. However, waveguide experiments are often based on optical pump pulses, which require treatment in a dynamic framework. In this paper, we present an effective Hamiltonian formalism in the dynamic regime using optical pulses that links waveguide optomechanics and cavity optomechanics, which can be used in the classical and quantum regime including quantum noise. Based on our formalism, a closed solution for coupled-mode equation under the undepleted assumption is provided and we found that the strong coupling regime is already accessible in current Brillouin waveguides by using pulses. We further investigate several possible experiments within waveguide optomechanics, including Brillouin-based coherent transfer, Brillouin cooling, and optoacoustic entanglement.
Contact
Research Group Birgit Stiller
Max Planck Institute for the Science of Light Staudtstr. 2 91058 Erlangen, Germany
